On-surface Ullmann polymerization via intermediate organometallic networks on Ag(111)

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چکیده

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On-surface Ullmann polymerization via intermediate organometallic networks on Ag(111).

The role of organometallic intermediates during on-surface polymerization via Ullmann coupling was studied on Ag(111). The polymerization progress was monitored by X-ray photoelectron spectroscopy (XPS). Scanning Tunneling Microscopy (STM) was used to characterize organometallic and covalent networks and to identify the temperature regimes for organometallic and covalent bond formation.

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’ Song comments on our recent paper, stating “it is apparent that the conclusion drawn from the XPS measurements and analysis is questionable, and the discussion of the XPS section was not well addressed”. In this reply, we show that while some of Song's comments are pertinent to certain technical aspects of photoelectron spectroscopy, most of his assumptions are unjustified and the critique as...

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Transition Metals Trigger On-Surface Ullmann Coupling Reaction: Intermediate, Catalyst and Template

In this chapter, we report on our recent studies of on-surface Ullmann coupling reaction and focus on the roles of the transition metals in the reaction. First, we discuss an organometallic intermediate state, which separates the reaction into two steps. Next, we examine the catalytic efficiency of Cu, Au, Ag, Pt, and Pd in the reaction. We analyze the bond formation yields when the reaction ta...

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Synthesis-in-place of highly-conjugated oligothiophene micropatterns via photo-activated Ullmann coupling on copper surface.

In contrast to the traditional thermally-activated Ullmann coupling, a photo-activated Ullmann coupling for facile synthesis of oligothiophene and polythiophene films and micropatterns is reported.

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ژورنال

عنوان ژورنال: Chem. Commun.

سال: 2014

ISSN: 1359-7345,1364-548X

DOI: 10.1039/c4cc02757d